WO1995017961A3 - Process for preparing a zeolite catalyst for the isomerizing of linear olefins to isoolefins - Google Patents

Process for preparing a zeolite catalyst for the isomerizing of linear olefins to isoolefins Download PDF

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Publication number
WO1995017961A3
WO1995017961A3 PCT/US1994/014861 US9414861W WO9517961A3 WO 1995017961 A3 WO1995017961 A3 WO 1995017961A3 US 9414861 W US9414861 W US 9414861W WO 9517961 A3 WO9517961 A3 WO 9517961A3
Authority
WO
WIPO (PCT)
Prior art keywords
isoolefins
isomerizing
linear olefins
pellet
preparing
Prior art date
Application number
PCT/US1994/014861
Other languages
French (fr)
Other versions
WO1995017961A2 (en
Inventor
Brendan Dermot Murray
Original Assignee
Shell Oil Co
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Priority to CA002180275A priority Critical patent/CA2180275C/en
Priority to DE69423241T priority patent/DE69423241T2/en
Priority to JP51815395A priority patent/JP3821841B2/en
Priority to AT95906108T priority patent/ATE189976T1/en
Priority to EP95906108A priority patent/EP0737102B1/en
Priority to BR9408441A priority patent/BR9408441A/en
Application filed by Shell Oil Co filed Critical Shell Oil Co
Priority to AU14450/95A priority patent/AU692215B2/en
Publication of WO1995017961A2 publication Critical patent/WO1995017961A2/en
Publication of WO1995017961A3 publication Critical patent/WO1995017961A3/en
Priority to FI962682A priority patent/FI962682A/en
Priority to NO19962769A priority patent/NO314248B1/en
Priority to NO20022242A priority patent/NO316443B1/en

Links

Classifications

    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/0009—Use of binding agents; Moulding; Pressing; Powdering; Granulating; Addition of materials ameliorating the mechanical properties of the product catalyst
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J29/00—Catalysts comprising molecular sieves
    • B01J29/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites
    • B01J29/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
    • B01J29/65—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the ferrierite type, e.g. types ZSM-21, ZSM-35 or ZSM-38, as exemplified by patent documents US4046859, US4016245 and US4046859, respectively
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C5/00—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms
    • C07C5/22—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms by isomerisation
    • C07C5/27—Rearrangement of carbon atoms in the hydrocarbon skeleton
    • C07C5/2767—Changing the number of side-chains
    • C07C5/277—Catalytic processes
    • C07C5/2775—Catalytic processes with crystalline alumino-silicates, e.g. molecular sieves
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2229/00—Aspects of molecular sieve catalysts not covered by B01J29/00
    • B01J2229/30—After treatment, characterised by the means used
    • B01J2229/42—Addition of matrix or binder particles
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2521/00—Catalysts comprising the elements, oxides or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium or hafnium
    • C07C2521/02—Boron or aluminium; Oxides or hydroxides thereof
    • C07C2521/04—Alumina
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2529/00—Catalysts comprising molecular sieves
    • C07C2529/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites, pillared clays
    • C07C2529/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2529/00—Catalysts comprising molecular sieves
    • C07C2529/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites, pillared clays
    • C07C2529/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
    • C07C2529/65—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the ferrierite type, e.g. types ZSM-21, ZSM-35 or ZSM-38
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2529/00—Catalysts comprising molecular sieves
    • C07C2529/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites, pillared clays
    • C07C2529/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
    • C07C2529/65—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the ferrierite type, e.g. types ZSM-21, ZSM-35 or ZSM-38
    • C07C2529/66—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the ferrierite type, e.g. types ZSM-21, ZSM-35 or ZSM-38 containing iron group metals, noble metals or copper
    • C07C2529/67—Noble metals

Abstract

An active and stable catalyst for isomerizing linear olefins to methyl branched isoolefins is provided by (a) mixing (i) a zeolite powder containing at least one zeolite with at least one one-dimensional pore structure having pore size small enough to retard by-product dimerization and coke formation and large enough to permit entry of the linear olefin and allow formation of the methyl branched isoolefin, (ii) an alumina-containing binder, (iii) water, (iv) at least one acid selected from monocarboxylic acids and inorganic acids and (v) at least one polycarboxylic acid; (b) forming a pellet of the mixture; and (c) calcining the pellet. The resulting catalyst has superior selectivity, higher maximum product concentration in the product stream and longer run length for isomerizing linear olefins to their corresponding isoolefins.
PCT/US1994/014861 1993-12-29 1994-12-23 Process for preparing a zeolite catalyst for the isomerizing of linear olefins to isoolefins WO1995017961A2 (en)

Priority Applications (10)

Application Number Priority Date Filing Date Title
DE69423241T DE69423241T2 (en) 1993-12-29 1994-12-23 METHOD FOR PRODUCING A ZEOLITE CATALYST FOR ISOMERIZING LINEAR OLEFINS TO IZOOLEFINS
JP51815395A JP3821841B2 (en) 1993-12-29 1994-12-23 Process for the preparation of zeolite catalysts for the isomerization of linear olefins to isoolefins
AT95906108T ATE189976T1 (en) 1993-12-29 1994-12-23 METHOD FOR PRODUCING A ZEOLITE CATALYST FOR THE ISOMERIZATION OF LINEAR OLEFINS TO IZOOLEFINS
EP95906108A EP0737102B1 (en) 1993-12-29 1994-12-23 Process for preparing a zeolite catalyst for the isomerizing of linear olefins to isoolefins
BR9408441A BR9408441A (en) 1993-12-29 1994-12-23 Process for preparing a zeolite catalyst for the isomerization of olefins to isoolefins
CA002180275A CA2180275C (en) 1993-12-29 1994-12-23 Process for preparing a zeolite catalyst for the isomerizing of linear olefins to isoolefins
AU14450/95A AU692215B2 (en) 1993-12-29 1994-12-23 Process for preparing a zeolite catalyst for the isomerizing of linear olefins to isoolefins
FI962682A FI962682A (en) 1993-12-29 1996-06-28 Process for the preparation of zeolite catalysts for the isomerization of linear olefins to isoolefins
NO19962769A NO314248B1 (en) 1993-12-29 1996-06-28 Process for the preparation of a zeolite catalyst for the isomerization of linear olefins to isoolefins, and a process of structural isomerization of a linear olefin
NO20022242A NO316443B1 (en) 1993-12-29 2002-05-10 Process of isomerization of olefins

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US175,004 1988-04-12
US08/175,004 US5510306A (en) 1993-12-29 1993-12-29 Process for isomerizing linear olefins to isoolefins

Publications (2)

Publication Number Publication Date
WO1995017961A2 WO1995017961A2 (en) 1995-07-06
WO1995017961A3 true WO1995017961A3 (en) 1995-09-28

Family

ID=22638436

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/US1994/014861 WO1995017961A2 (en) 1993-12-29 1994-12-23 Process for preparing a zeolite catalyst for the isomerizing of linear olefins to isoolefins

Country Status (18)

Country Link
US (3) US5510306A (en)
EP (2) EP0854125B1 (en)
JP (2) JP3821841B2 (en)
KR (1) KR100370512B1 (en)
CN (2) CN1079286C (en)
AT (2) ATE251098T1 (en)
AU (1) AU692215B2 (en)
BR (1) BR9408441A (en)
CA (1) CA2180275C (en)
DE (2) DE69423241T2 (en)
ES (1) ES2208990T3 (en)
FI (1) FI962682A (en)
MY (1) MY121924A (en)
NO (2) NO314248B1 (en)
SG (1) SG64913A1 (en)
TW (1) TW289740B (en)
WO (1) WO1995017961A2 (en)
ZA (1) ZA9410398B (en)

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