WO2004013095A3 - Catalyst for aromatization of alkanes, process of making and using thereof - Google Patents
Catalyst for aromatization of alkanes, process of making and using thereof Download PDFInfo
- Publication number
- WO2004013095A3 WO2004013095A3 PCT/US2003/024314 US0324314W WO2004013095A3 WO 2004013095 A3 WO2004013095 A3 WO 2004013095A3 US 0324314 W US0324314 W US 0324314W WO 2004013095 A3 WO2004013095 A3 WO 2004013095A3
- Authority
- WO
- WIPO (PCT)
- Prior art keywords
- catalyst
- aromatization
- alkanes
- platinum
- germanium
- Prior art date
Links
- 239000003054 catalyst Substances 0.000 title abstract 12
- 238000000034 method Methods 0.000 title abstract 5
- 238000005899 aromatization reaction Methods 0.000 title abstract 4
- 150000001335 aliphatic alkanes Chemical class 0.000 title abstract 3
- BASFCYQUMIYNBI-UHFFFAOYSA-N platinum Chemical compound [Pt] BASFCYQUMIYNBI-UHFFFAOYSA-N 0.000 abstract 7
- UHOVQNZJYSORNB-UHFFFAOYSA-N Benzene Chemical compound C1=CC=CC=C1 UHOVQNZJYSORNB-UHFFFAOYSA-N 0.000 abstract 3
- VYPSYNLAJGMNEJ-UHFFFAOYSA-N Silicium dioxide Chemical compound O=[Si]=O VYPSYNLAJGMNEJ-UHFFFAOYSA-N 0.000 abstract 3
- YXFVVABEGXRONW-UHFFFAOYSA-N Toluene Chemical compound CC1=CC=CC=C1 YXFVVABEGXRONW-UHFFFAOYSA-N 0.000 abstract 3
- 229910021536 Zeolite Inorganic materials 0.000 abstract 3
- HNPSIPDUKPIQMN-UHFFFAOYSA-N dioxosilane;oxo(oxoalumanyloxy)alumane Chemical compound O=[Si]=O.O=[Al]O[Al]=O HNPSIPDUKPIQMN-UHFFFAOYSA-N 0.000 abstract 3
- 229910052697 platinum Inorganic materials 0.000 abstract 3
- 239000010457 zeolite Substances 0.000 abstract 3
- CPLXHLVBOLITMK-UHFFFAOYSA-N Magnesium oxide Chemical compound [Mg]=O CPLXHLVBOLITMK-UHFFFAOYSA-N 0.000 abstract 2
- ATUOYWHBWRKTHZ-UHFFFAOYSA-N Propane Chemical compound CCC ATUOYWHBWRKTHZ-UHFFFAOYSA-N 0.000 abstract 2
- GWEVSGVZZGPLCZ-UHFFFAOYSA-N Titan oxide Chemical compound O=[Ti]=O GWEVSGVZZGPLCZ-UHFFFAOYSA-N 0.000 abstract 2
- MCMNRKCIXSYSNV-UHFFFAOYSA-N Zirconium dioxide Chemical compound O=[Zr]=O MCMNRKCIXSYSNV-UHFFFAOYSA-N 0.000 abstract 2
- 229910052732 germanium Inorganic materials 0.000 abstract 2
- GNPVGFCGXDBREM-UHFFFAOYSA-N germanium atom Chemical compound [Ge] GNPVGFCGXDBREM-UHFFFAOYSA-N 0.000 abstract 2
- 150000003464 sulfur compounds Chemical class 0.000 abstract 2
- ZOXJGFHDIHLPTG-UHFFFAOYSA-N Boron Chemical group [B] ZOXJGFHDIHLPTG-UHFFFAOYSA-N 0.000 abstract 1
- 239000004215 Carbon black (E152) Substances 0.000 abstract 1
- GYHNNYVSQQEPJS-UHFFFAOYSA-N Gallium Chemical group [Ga] GYHNNYVSQQEPJS-UHFFFAOYSA-N 0.000 abstract 1
- CTQNGGLPUBDAKN-UHFFFAOYSA-N O-Xylene Chemical compound CC1=CC=CC=C1C CTQNGGLPUBDAKN-UHFFFAOYSA-N 0.000 abstract 1
- ATJFFYVFTNAWJD-UHFFFAOYSA-N Tin Chemical group [Sn] ATJFFYVFTNAWJD-UHFFFAOYSA-N 0.000 abstract 1
- RTAQQCXQSZGOHL-UHFFFAOYSA-N Titanium Chemical group [Ti] RTAQQCXQSZGOHL-UHFFFAOYSA-N 0.000 abstract 1
- 229910052782 aluminium Inorganic materials 0.000 abstract 1
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical group [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 abstract 1
- PNEYBMLMFCGWSK-UHFFFAOYSA-N aluminium oxide Inorganic materials [O-2].[O-2].[O-2].[Al+3].[Al+3] PNEYBMLMFCGWSK-UHFFFAOYSA-N 0.000 abstract 1
- -1 aluminum-silicongermanium Chemical group 0.000 abstract 1
- 229910052796 boron Inorganic materials 0.000 abstract 1
- 125000004432 carbon atom Chemical group C* 0.000 abstract 1
- 150000001768 cations Chemical class 0.000 abstract 1
- 229910052733 gallium Inorganic materials 0.000 abstract 1
- PCHJSUWPFVWCPO-UHFFFAOYSA-N gold Chemical compound [Au] PCHJSUWPFVWCPO-UHFFFAOYSA-N 0.000 abstract 1
- 229910052737 gold Inorganic materials 0.000 abstract 1
- 239000010931 gold Substances 0.000 abstract 1
- 229930195733 hydrocarbon Natural products 0.000 abstract 1
- 150000002430 hydrocarbons Chemical class 0.000 abstract 1
- 229910052738 indium Inorganic materials 0.000 abstract 1
- APFVFJFRJDLVQX-UHFFFAOYSA-N indium atom Chemical group [In] APFVFJFRJDLVQX-UHFFFAOYSA-N 0.000 abstract 1
- 239000000395 magnesium oxide Substances 0.000 abstract 1
- 239000000203 mixture Substances 0.000 abstract 1
- 229910000510 noble metal Inorganic materials 0.000 abstract 1
- 239000001294 propane Substances 0.000 abstract 1
- 239000000377 silicon dioxide Substances 0.000 abstract 1
- 229910052714 tellurium Inorganic materials 0.000 abstract 1
- PORWMNRCUJJQNO-UHFFFAOYSA-N tellurium atom Chemical group [Te] PORWMNRCUJJQNO-UHFFFAOYSA-N 0.000 abstract 1
- ZCUFMDLYAMJYST-UHFFFAOYSA-N thorium dioxide Chemical compound O=[Th]=O ZCUFMDLYAMJYST-UHFFFAOYSA-N 0.000 abstract 1
- 229910052718 tin Inorganic materials 0.000 abstract 1
- 239000010936 titanium Substances 0.000 abstract 1
- 229910052719 titanium Inorganic materials 0.000 abstract 1
- 239000008096 xylene Substances 0.000 abstract 1
Classifications
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- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C2/00—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J29/00—Catalysts comprising molecular sieves
- B01J29/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J29/00—Catalysts comprising molecular sieves
- B01J29/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites
- B01J29/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
- B01J29/064—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof containing iron group metals, noble metals or copper
- B01J29/068—Noble metals
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J29/00—Catalysts comprising molecular sieves
- B01J29/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites
- B01J29/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
- B01J29/40—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the pentasil type, e.g. types ZSM-5, ZSM-8 or ZSM-11, as exemplified by patent documents US3702886, GB1334243 and US3709979, respectively
- B01J29/42—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the pentasil type, e.g. types ZSM-5, ZSM-8 or ZSM-11, as exemplified by patent documents US3702886, GB1334243 and US3709979, respectively containing iron group metals, noble metals or copper
- B01J29/44—Noble metals
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C2/00—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms
- C07C2/76—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms by condensation of hydrocarbons with partial elimination of hydrogen
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2229/00—Aspects of molecular sieve catalysts not covered by B01J29/00
- B01J2229/10—After treatment, characterised by the effect to be obtained
- B01J2229/18—After treatment, characterised by the effect to be obtained to introduce other elements into or onto the molecular sieve itself
- B01J2229/186—After treatment, characterised by the effect to be obtained to introduce other elements into or onto the molecular sieve itself not in framework positions
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
- C07C2523/14—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of germanium, tin or lead
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
- C07C2523/38—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of noble metals
- C07C2523/40—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of noble metals of the platinum group metals
- C07C2523/42—Platinum
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C2527/00—Catalysts comprising the elements or compounds of halogens, sulfur, selenium, tellurium, phosphorus or nitrogen; Catalysts comprising carbon compounds
- C07C2527/02—Sulfur, selenium or tellurium; Compounds thereof
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C2529/00—Catalysts comprising molecular sieves
- C07C2529/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites, pillared clays
- C07C2529/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
- C07C2529/70—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of types characterised by their specific structure not provided for in groups C07C2529/08 - C07C2529/65
- C07C2529/72—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of types characterised by their specific structure not provided for in groups C07C2529/08 - C07C2529/65 containing iron group metals, noble metals or copper
- C07C2529/74—Noble metals
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
- Y02P20/00—Technologies relating to chemical industry
- Y02P20/50—Improvements relating to the production of bulk chemicals
- Y02P20/52—Improvements relating to the production of bulk chemicals using catalysts, e.g. selective catalysts
Abstract
Priority Applications (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
EP03767135.1A EP1531931B1 (en) | 2002-08-06 | 2003-08-05 | Catalyst for aromatization of alkanes, process of making and using thereof |
AU2003258030A AU2003258030A1 (en) | 2002-08-06 | 2003-08-05 | Catalyst for aromatization of alkanes, process of making and using thereof |
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
US10/213,313 | 2002-08-06 | ||
US10/213,313 US6784333B2 (en) | 2002-08-06 | 2002-08-06 | Catalyst for aromatization of alkanes, process of making and using thereof |
Publications (2)
Publication Number | Publication Date |
---|---|
WO2004013095A2 WO2004013095A2 (en) | 2004-02-12 |
WO2004013095A3 true WO2004013095A3 (en) | 2004-07-08 |
Family
ID=31494438
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
PCT/US2003/024314 WO2004013095A2 (en) | 2002-08-06 | 2003-08-05 | Catalyst for aromatization of alkanes, process of making and using thereof |
Country Status (6)
Country | Link |
---|---|
US (2) | US6784333B2 (en) |
EP (1) | EP1531931B1 (en) |
CN (1) | CN100422122C (en) |
AU (1) | AU2003258030A1 (en) |
RU (1) | RU2307117C2 (en) |
WO (1) | WO2004013095A2 (en) |
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US7745675B2 (en) * | 2006-12-20 | 2010-06-29 | Saudi Basic Industries Corporation | Regeneration of platinum-germanium zeolite catalyst |
US7906696B2 (en) * | 2007-01-22 | 2011-03-15 | Saudi Basic Industries Corporation | Process of using zeolite catalyst for hydrocarbon conversion |
US7902413B2 (en) | 2007-04-12 | 2011-03-08 | Saudi Basic Industries Corporation | Aromatization of alkanes using a germanium-zeolite catalyst |
US8969232B2 (en) * | 2007-05-24 | 2015-03-03 | Saudi Basic Industries Corporation | Catalyst for conversion of hydrocarbons, process of making and process of using thereof—incorporation 2 |
US9221723B2 (en) * | 2007-05-24 | 2015-12-29 | Saudi Basic Industries Corporation | Catalyst for conversion of hydrocarbons, process of making and process of using thereof—incorporation-1 |
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WO2009076393A2 (en) * | 2007-12-12 | 2009-06-18 | Shell Oil Company | Process for the conversion of ethane or mixed lower alkanes to aromatic hydrocarbons |
US8809608B2 (en) * | 2008-02-18 | 2014-08-19 | Shell Oil Company | Process for the conversion of lower alkanes to aromatic hydrocarbons |
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US8153852B2 (en) * | 2009-04-29 | 2012-04-10 | Saudi Basic Industries Corporation | Process of using germanium zeolite catalyst for alkane aromatization |
CN102548657B (en) * | 2009-09-30 | 2015-01-21 | 埃克森美孚化学专利公司 | Production of aromatics from methane |
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US20110132804A1 (en) * | 2009-12-04 | 2011-06-09 | Saudi Basic Industries Corporation | Increasing octane number of light naphtha using a germanium-zeolite catalyst |
WO2011143306A2 (en) | 2010-05-12 | 2011-11-17 | Shell Oil Company | Process for the conversion of lower alkanes to aromatic hydrocarbons |
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US10987661B2 (en) | 2011-02-17 | 2021-04-27 | AMG Chemistry and Catalysis Consulting, LLC | Alloyed zeolite catalyst component, method for making and catalytic application thereof |
US9242233B2 (en) | 2012-05-02 | 2016-01-26 | Saudi Basic Industries Corporation | Catalyst for light naphtha aromatization |
US8772192B2 (en) | 2012-06-29 | 2014-07-08 | Saudi Basic Industries Corporation | Germanium silicalite catalyst and method of preparation and use |
US9352306B2 (en) * | 2012-07-03 | 2016-05-31 | Basf Se | Catalyst and process for removing oxygen from hydrocarbon streams |
US9180441B2 (en) | 2012-09-20 | 2015-11-10 | Saudi Basic Industries Corporation | Method of forming zeolite shaped body with silica binder |
CN103934016B (en) * | 2013-01-23 | 2016-08-17 | 中国石油化工股份有限公司 | Mo/ molecular sieve carried type method for preparing catalyst |
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JP3191489B2 (en) * | 1993-05-27 | 2001-07-23 | 三菱化学株式会社 | Method for producing halogenated phthalic anhydride |
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-
2002
- 2002-08-06 US US10/213,313 patent/US6784333B2/en not_active Expired - Lifetime
-
2003
- 2003-08-05 RU RU2005102841/04A patent/RU2307117C2/en active
- 2003-08-05 EP EP03767135.1A patent/EP1531931B1/en not_active Expired - Fee Related
- 2003-08-05 AU AU2003258030A patent/AU2003258030A1/en not_active Abandoned
- 2003-08-05 CN CNB038189828A patent/CN100422122C/en not_active Expired - Fee Related
- 2003-08-05 WO PCT/US2003/024314 patent/WO2004013095A2/en not_active Application Discontinuation
-
2004
- 2004-03-31 US US10/814,913 patent/US7247593B2/en not_active Expired - Lifetime
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US4704494A (en) * | 1984-08-15 | 1987-11-03 | Showa Shell Sekiyu Kabushiki Kaisha | Conversion process of aromatic hydrocarbon from low molecular paraffin hydrocarbon |
US4590323A (en) * | 1985-06-12 | 1986-05-20 | Mobil Oil Corporation | Conversion of paraffins to aromatics over zeolites modified with oxides of group IIIA, IVA and VA elements |
US5371307A (en) * | 1988-04-01 | 1994-12-06 | Rhone-Poulenc Chimie | Silica/germanium oxide zeolites |
Also Published As
Publication number | Publication date |
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AU2003258030A8 (en) | 2004-02-23 |
AU2003258030A1 (en) | 2004-02-23 |
CN1674988A (en) | 2005-09-28 |
EP1531931A2 (en) | 2005-05-25 |
US20040028584A1 (en) | 2004-02-12 |
RU2005102841A (en) | 2005-07-10 |
US7247593B2 (en) | 2007-07-24 |
WO2004013095A2 (en) | 2004-02-12 |
US20040192539A1 (en) | 2004-09-30 |
EP1531931B1 (en) | 2019-01-16 |
RU2307117C2 (en) | 2007-09-27 |
EP1531931A4 (en) | 2012-03-21 |
CN100422122C (en) | 2008-10-01 |
US6784333B2 (en) | 2004-08-31 |
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