WO2006086457A3 - Palladium-cobalt particles as oxygen-reduction electrocatalysts - Google Patents

Palladium-cobalt particles as oxygen-reduction electrocatalysts Download PDF

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Publication number
WO2006086457A3
WO2006086457A3 PCT/US2006/004402 US2006004402W WO2006086457A3 WO 2006086457 A3 WO2006086457 A3 WO 2006086457A3 US 2006004402 W US2006004402 W US 2006004402W WO 2006086457 A3 WO2006086457 A3 WO 2006086457A3
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WIPO (PCT)
Prior art keywords
palladium
oxygen
cobalt particles
electrocatalysts
relates
Prior art date
Application number
PCT/US2006/004402
Other languages
French (fr)
Other versions
WO2006086457A2 (en
Inventor
Radoslav R Adzic
Tao Huang
Original Assignee
Brookhaven Science Ass Llc
Radoslav R Adzic
Tao Huang
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Application filed by Brookhaven Science Ass Llc, Radoslav R Adzic, Tao Huang filed Critical Brookhaven Science Ass Llc
Priority to MX2007009666A priority Critical patent/MX2007009666A/en
Priority to JP2007555187A priority patent/JP5443691B2/en
Priority to CA2596433A priority patent/CA2596433C/en
Priority to EP06734564A priority patent/EP1849201B1/en
Priority to KR1020077020321A priority patent/KR101310946B1/en
Priority to CN2006800045735A priority patent/CN101151745B/en
Publication of WO2006086457A2 publication Critical patent/WO2006086457A2/en
Publication of WO2006086457A3 publication Critical patent/WO2006086457A3/en

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    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90Selection of catalytic material
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1009Fuel cells with solid electrolytes with one of the reactants being liquid, solid or liquid-charged
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90Selection of catalytic material
    • H01M4/9041Metals or alloys
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90Selection of catalytic material
    • H01M4/9075Catalytic material supported on carriers, e.g. powder carriers
    • H01M4/9083Catalytic material supported on carriers, e.g. powder carriers on carbon or graphite
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90Selection of catalytic material
    • H01M4/92Metals of platinum group
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90Selection of catalytic material
    • H01M4/92Metals of platinum group
    • H01M4/921Alloys or mixtures with metallic elements
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90Selection of catalytic material
    • H01M4/92Metals of platinum group
    • H01M4/925Metals of platinum group supported on carriers, e.g. powder carriers
    • H01M4/926Metals of platinum group supported on carriers, e.g. powder carriers on carbon or graphite
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/96Carbon-based electrodes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/04Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1009Fuel cells with solid electrolytes with one of the reactants being liquid, solid or liquid-charged
    • H01M8/1011Direct alcohol fuel cells [DAFC], e.g. direct methanol fuel cells [DMFC]
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B82NANOTECHNOLOGY
    • B82YSPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES; MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES; MANUFACTURE OR TREATMENT OF NANOSTRUCTURES
    • B82Y30/00Nanotechnology for materials or surface science, e.g. nanocomposites
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M2008/1095Fuel cells with polymeric electrolytes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8647Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites
    • H01M4/8652Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites as mixture
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8647Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites
    • H01M4/8657Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites layered
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Catalysts (AREA)
  • Manufacture Of Metal Powder And Suspensions Thereof (AREA)
  • Inert Electrodes (AREA)
  • Powder Metallurgy (AREA)
  • Fuel Cell (AREA)

Abstract

The present invention relates to palladium-cobalt particles useful as oxygen- reducing electrocatalysts. The invention also relates to oxygen-reducing cathodes and fuel cells containing these palladium-cobalt particles. The invention additionally relates to methods for the production of electrical energy by using the palladium- cobalt particles of the invention.
PCT/US2006/004402 2005-02-10 2006-02-09 Palladium-cobalt particles as oxygen-reduction electrocatalysts WO2006086457A2 (en)

Priority Applications (6)

Application Number Priority Date Filing Date Title
MX2007009666A MX2007009666A (en) 2005-02-10 2006-02-09 Palladium-cobalt particles as oxygen-reduction electrocatalysts.
JP2007555187A JP5443691B2 (en) 2005-02-10 2006-02-09 Palladium-cobalt particles as oxygen reduction electrocatalysts
CA2596433A CA2596433C (en) 2005-02-10 2006-02-09 Palladium-cobalt particles as oxygen-reduction electrocatalysts
EP06734564A EP1849201B1 (en) 2005-02-10 2006-02-09 Palladium-cobalt particles as oxygen-reduction electrocatalysts
KR1020077020321A KR101310946B1 (en) 2005-02-10 2006-02-09 Palladium-Cobalt Particles as Oxygen-Reduction Electrocatalysts
CN2006800045735A CN101151745B (en) 2005-02-10 2006-02-09 Palladium-cobalt particles as oxygen-reduction electrocatalysts

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US11/054,587 2005-02-10
US11/054,587 US7632601B2 (en) 2005-02-10 2005-02-10 Palladium-cobalt particles as oxygen-reduction electrocatalysts

Publications (2)

Publication Number Publication Date
WO2006086457A2 WO2006086457A2 (en) 2006-08-17
WO2006086457A3 true WO2006086457A3 (en) 2007-09-07

Family

ID=36780345

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PCT/US2006/004402 WO2006086457A2 (en) 2005-02-10 2006-02-09 Palladium-cobalt particles as oxygen-reduction electrocatalysts

Country Status (9)

Country Link
US (1) US7632601B2 (en)
EP (1) EP1849201B1 (en)
JP (2) JP5443691B2 (en)
KR (1) KR101310946B1 (en)
CN (1) CN101151745B (en)
CA (1) CA2596433C (en)
MX (1) MX2007009666A (en)
RU (1) RU2394311C2 (en)
WO (1) WO2006086457A2 (en)

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US7632601B2 (en) * 2005-02-10 2009-12-15 Brookhaven Science Associates, Llc Palladium-cobalt particles as oxygen-reduction electrocatalysts
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US20080152992A1 (en) * 2006-12-20 2008-06-26 Canon Kabushiki Kaisha Constituent member for membrane electrode assembly, membrane electrode assembly, polymer electrolyte fuel cell, and method for producing constituent member and membrane electrode assembly
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Publication number Publication date
CN101151745A (en) 2008-03-26
US7632601B2 (en) 2009-12-15
CA2596433C (en) 2013-12-31
KR20070100846A (en) 2007-10-11
EP1849201A4 (en) 2009-07-29
CA2596433A1 (en) 2006-08-17
RU2007133730A (en) 2009-03-20
MX2007009666A (en) 2007-10-02
JP2013243154A (en) 2013-12-05
KR101310946B1 (en) 2013-09-23
RU2394311C2 (en) 2010-07-10
EP1849201A2 (en) 2007-10-31
CN101151745B (en) 2011-06-15
JP2008533654A (en) 2008-08-21
US20060177728A1 (en) 2006-08-10
WO2006086457A2 (en) 2006-08-17
EP1849201B1 (en) 2012-05-30
JP5443691B2 (en) 2014-03-19

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